Direct Casting Techniques - Temperature Induced Forming

 

Direct Casting Techniques are based on constant volume, i.e. the gelation of a liquified slurry is achieved without removal of the dispersing agent (e.g. water). Ceramic particle suspensions with high solids loading (>60 vol.%) are poured into dense molds and solidified by changing the colloidal stability. In this way complex-shaped ceramic green bodies can be achieved. My group in collaboration with Prof. Aldinger from the Max-Planck-Institute for Metals Research in Germany introduced one of the simplest direct casting techniques that is based on commercially available inexpensive compounds. This technique is referred to as Temperature Induced Forming (TIF) since the coagulation of a dispersed slurry is induced via a mild increase in temperature.  The technique is based on a combination of fundamental science from solution chemistry and colloid stability.

This novel direct casting technique has been successfully applied to alumina, zirconia, and mullite powder systems, zirconia-toughened-alumina, zirconia-toughened-mullite, yttria-stabilized-zirconia binary ceramic powder systems, and yttiria-magnesia-stabilized-zirconia ternary ceramic system. We study the rheological behavior of the casting slips and developed a novel concept to quantitatively predict the gelation and wet green strength of a gelled body via a combination of percolation and crystallization theories.

 

 

Publications

  1. Yunpeng Yang and Wolfgang M. Sigmund, “Preparation, Characterization, and Gelation of Temperature-Induced Forming (TIF) Alumina Slurries,” Journal of Materials Synthesis and Processing, 9 [2] (2001) 103-109.
  2. Yunpeng Yang and Wolfgang M. Sigmund, “Effect of Particle Volume Fraction on the Gelation Behavior of the Temperature Induced Forming (TIF) Aqueous Alumina Suspensions,” J. Am. Ceram. Soc., 84 [9] (2001) 2138-40.
  3. Yunpeng Yang and Wolfgang M. Sigmund, “Estimation of the Volume Fraction Gelation Threshold for the Temperature Induced Forming (TIF) Alumina Aqueous Suspensions Using Rheological Measurement,” Journal of Ceramic Processing Research, 2 [3] (2001) 120-124.
  4. Yunpeng Yang and Wolfgang M. Sigmund, “Effect of calcium ion addition on dispersant adsorption in temperature induced forming (TIF) alumina slurry,” J. Mater. Sci. Lett., 20 (2001) 651-653.
  5. Yunpeng Yang and Wolfgang M. Sigmund, “Percolation Theory Model for the Temperature Induced Forming (TIF) Ceramic Slurries, Part I – Theoretical Calculations,” submitted to J. Europ. Ceram. Soc., (2001).
  6. Yunpeng Yang and Wolfgang M. Sigmund, “Percolation Theory Model for the Temperature Induced Forming (TIF) Ceramic Slurries, Part II – Experimental Derivations of the Equation Parameters,” submitted to J. Europ. Ceram. Soc., (2001).